Stream sediment geochemical data for 21282 samples from a regional sampling program in the Kimberley region of Western Australia have been acquired in digital form. The samples were collected and analysed by Kimberley Ventures, Pickands Mather and Company International Managing Agents in 1964, with additional analysis carried out in subsequent years. The stream sediment samples comprise the -80 mesh (i.e. less than 177 micron) fraction. Details of the sampling program, and analytical techniques for all but Cobalt (Co) are contained in the Annual Report for 1964, available in open file from DoIR as A439 (M67, I251A)